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A Diiron Hydrogenase Mimic Featuring a 1,2,3-Triazolylidene

Abstract : A novel complex featuring a mesoionic carbene [Fe2(CO)5(trz)(μ-pdt)] (1) (trz = 1-phenyl-l,3-methyl,4-butyl-1,2,3-triazol-5-ylidene), was synthesized and spectroscopically and structurally characterized. The reduc-tive behaviour of this compound in the presence and in the absence of acid (CH3CO2H) was examined by cyclic voltammetry (CV) that revealed the lack of efficient activity towards proton reduction
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Submitted on : Monday, July 20, 2020 - 3:10:47 PM
Last modification on : Monday, October 11, 2021 - 2:22:08 PM

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Andrea Mele, Simone Bertini, Martin Albrecht, Catherine Elleouet, François Pétillon, et al.. A Diiron Hydrogenase Mimic Featuring a 1,2,3-Triazolylidene. CHIMIA, Schweizerische Chemische Gesellschaft, 2020, 74 (6), pp.499-503. ⟨10.2533/chimia.2020.499⟩. ⟨hal-02902975⟩



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